Natural language has been extensively used for modeling text-attributed graphs with LLMs. Natural language is used to describe the graph for LLMs to understand or serve as component of the graph, e.g., textual attributes for embedding generation. However, natural language is inherently redundant and unstructured, making it unsuitable for modeling high-order neighbors with LLMs. Specifically, (i) graph descriptions become verbose, overwhelming LLMs, and (ii) only relying on attribute embeddings limits LLM’s ability to capture the adequate graph structural information. These limitations make it difficult to model graphs both concisely and adequately using sole natural language with LLMs.Inspired by the observation that LLMs pre-trained on one language can achieve exceptional performance on another with minimal additional training, we propose Graph-Defined Language for Large Language Model (GDL4LLM). This novel framework enables LLMs to transfer their powerful language understanding capabilities to graph-structured data. GDL4LLM translates the graph into a graph language corpus instead of graph descriptions and pre-trains LLMs on this corpus to adequately understand the graph. This corpus represents the subgraph centered around target nodes concisely with only a few tokens during fine-tuning on downstream tasks. By treating the graph as a new language, GDL4LLM enables LLMs to model text-attributed graph adequately and concisely. Extensive experiments on five datasets demonstrate that GDL4LLM outperforms description-based and embedding-based baselines by efficiently modeling different orders of neighbors.