Traditional tabular data synthesis methods often overlook the cross-modal heterogeneity of real-world tables, where structured continuous and discrete attributes coexist with unstructured long-text columns. Existing synthesis approaches struggle to simultaneously achieve accurate statistical fidelity for non-textual attributes and consistent semantic constraints between textual and non-textual attributes. In this work, we establish the first benchmark for long-text tabular data synthesis and introduce a novel metric, termed Textual Column Correlation Fidelity (TCCF), to quantify cross-modal semantic alignment. We propose AFT-Tab, an adversarial fine-tuning framework that synergistically trains an LLM-based text generator and a deep-learning-based non-textual generator. Through a dual-feedback mechanism guided by an LLM discriminator, AFT-Tab ensures both precise statistical distributions and rigorous semantic constraints. Experimental results show that AFT-Tab significantly outperforms state-of-the-art baselines in statistical fidelity, TCCF, diversity, and downstream task utility.