Binary quantization represents the most extreme form of compression, reducing weights to ±1 for maximal memory and computational efficiency. While recent sparsity-aware binarization achieves sub-1-bit compression via weight pruning, it faces critical challenger: performance degradation, mask-management overhead, and limited hardware compatibility. In this paper, we present BTC-LLM, a novel sub-1-bit LLM quantization framework that leverages binary pattern clustering and weight transformation to overcome these limitations. Our approach incorporates two key innovations: (1) a Binary Codebook that clusters recurring vectors into compact indices using custom distance metrics and sign-based updates; (2) a Learnable Transformation that reduces outliers and promotes shared sign patterns among binary weights. This eliminates sparse masks, enabling efficient inference on standard hardware. Extensive evaluations across LLaMA, Qwen, and FBI-LLM families demonstrate that BTC-LLM achieves state-of-the-art results in extreme compression (1.11–0.7 bits). Notably, BTC-LLM compressed to 0.8 bits on LLaMA-2-13B maintains high performance—with only a 3.1% accuracy drop in zero-shot benchmarks—while delivering a 1.6× speedup over FP16.

Large language model (LLM) reinforcement learning (RL) pipelines are often bottlenecked by rollout generation, making end-to-end training slow. Recent work mitigates this by running rollouts with quantization to accelerate decoding, which is the most expensive stage of the RL loop. However, these setups destabilize optimization by amplifying the training–-inference gap: rollouts are operated at low precision, while learning updates are computed at full precision. To address this challenge, we propose QaRL (Rollout Alignment Quantization-Aware RL), which aligns training-side forward with the quantized rollout to minimize mismatch. We further identify a failure mode in quantized rollouts: long-form responses tend to produce repetitive, garbled tokens (error tokens). To mitigate these problems, we introduce TBPO (Trust-Band Policy Optimization), a sequence-level objective with dual clipping for negative samples, aimed to keep updates within the trust region. On Qwen3-30B-A3B MoE for math problems, QaRL outperforms quantized-rollout training by +5.5 while improving stability and preserving low-bit throughput benefits.